Issue

Vol. 16 (2024)

Lightweight Dual-Functional Segregated Nanocomposite Foams for Integrated Infrared Stealth and Absorption-Dominant Electromagnetic Interference Shielding

https://doi.org/10.1007/s40820-024-01450-0
Zhonglei Ma
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Ruochu Jiang
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Jiayao Jing
College of Chemistry and Chemical Engineering, Key Laboratory of Auxiliary Chemistry and Technology for Chemical Industry, Ministry of Education, Shaanxi University of Science and Technology, Xi’an 710072, People’s Republic of China
Songlei Kang
College of Chemistry and Chemical Engineering, Key Laboratory of Auxiliary Chemistry and Technology for Chemical Industry, Ministry of Education, Shaanxi University of Science and Technology, Xi’an 710072, People’s Republic of China
Li Ma
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada
Kefan Zhang
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Junxian Li
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Yu Zhang
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Jianbin Qin
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Shuhuan Yun
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Guangcheng Zhang
MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions, Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China

Corresponding Author: Guangcheng Zhang

zhangguc@nwpu.edu.cn

Nano-Micro Letters, Vol. 16 (2024), Article Number: 223

Abstract

Lightweight infrared stealth and absorption-dominant electromagnetic interference (EMI) shielding materials are highly desirable in areas of aerospace, weapons, military and wearable electronics. Herein, lightweight and high-efficiency dual-functional segregated nanocomposite foams with microcellular structures are developed for integrated infrared stealth and absorption-dominant EMI shielding via the efficient and scalable supercritical CO2 (SC-CO2) foaming combined with hydrogen bonding assembly and compression molding strategy. The obtained lightweight segregated nanocomposite foams exhibit superior infrared stealth performances benefitting from the synergistic effect of highly effective thermal insulation and low infrared emissivity, and outstanding absorption-dominant EMI shielding performances attributed to the synchronous construction of microcellular structures and segregated structures. Particularly, the segregated nanocomposite foams present a large radiation temperature reduction of 70.2 °C at the object temperature of 100 °C, and a significantly improved EM wave absorptivity/reflectivity (A/R) ratio of 2.15 at an ultralow Ti3C2Tx content of 1.7 vol%. Moreover, the segregated nanocomposite foams exhibit outstanding working reliability and stability upon dynamic compression cycles. The results demonstrate that the lightweight and high-efficiency dual-functional segregated nanocomposite foams have excellent potentials for infrared stealth and absorption-dominant EMI shielding applications in aerospace, weapons, military and wearable electronics.


Highlights:
1 Lightweight dual-functional segregated nanocomposite foams are developed via the supercritical CO2 (SC-CO2) foaming combined with hydrogen bonding assembly and compression molding strategy
2 The segregated nanocomposite foams exhibit superior infrared stealth performances benefitting from the synergistic effect of highly effective thermal insulation and low infrared emissivity.
3 Excellent absorption-dominant electromagnetic interference shielding performances are achieved owing to the synchronous construction of microcellular structures and segregated structures

Keywords

Segregated nanocomposite foams Microcellular structures Infrared stealth EMI shielding Low infrared emissivity
Ma, Zhonglei, Ruochu Jiang, Jiayao Jing, Songlei Kang, Li Ma, Kefan Zhang, Junxian Li, Yu Zhang, Jianbin Qin, Shuhuan Yun, and Guangcheng Zhang. 2024. “Lightweight Dual-Functional Segregated Nanocomposite Foams for Integrated Infrared Stealth and Absorption-Dominant Electromagnetic Interference Shielding”. Nano-Micro Letters 16 (June):223. https://doi.org/10.1007/s40820-024-01450-0.
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