Issue

Vol. 15 (2023)

Multifunctional Perovskite Photodetectors: From Molecular-Scale Crystal Structure Design to Micro/Nano-scale Morphology Manipulation

https://doi.org/10.1007/s40820-023-01161-y
Yingjie Zhao
College of Chemistry, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Xing Yin
College of Chemistry, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Pengwei Li
College of Chemistry, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Ziqiu Ren
Henan Institute of Advanced Technology, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Zhenkun Gu
Henan Institute of Advanced Technology, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Yiqiang Zhang
College of Chemistry, Zhengzhou University, Zhengzhou 450001, People’s Republic of China
Yanlin Song
College of Chemistry, Zhengzhou University, Zhengzhou 450001, People’s Republic of China

Corresponding Author: Yanlin Song

ylsong@iccas.ac.cn

Nano-Micro Letters, Vol. 15 (2023), Article Number: 187

Abstract

Multifunctional photodetectors boost the development of traditional optical communication technology and emerging artificial intelligence fields, such as robotics and autonomous driving. However, the current implementation of multifunctional detectors is based on the physical combination of optical lenses, gratings, and multiple photodetectors, the large size and its complex structure hinder the miniaturization, lightweight, and integration of devices. In contrast, perovskite materials have achieved remarkable progress in the field of multifunctional photodetectors due to their diverse crystal structures, simple morphology manipulation, and excellent optoelectronic properties. In this review, we first overview the crystal structures and morphology manipulation techniques of perovskite materials and then summarize the working mechanism and performance parameters of multifunctional photodetectors. Furthermore, the fabrication strategies of multifunctional perovskite photodetectors and their advancements are highlighted, including polarized light detection, spectral detection, angle-sensing detection, and self-powered detection. Finally, the existing problems of multifunctional detectors and the perspectives of their future development are presented.


Highlights:
1 Multidimensional detection of intensity, wavelength, polarization, and angle of the incidence light significantly accelerates the development of optical information technology and artificial intelligence fields.
2 The first comprehensive overview of the advancement of multifunctional photodetectors for perovskite semiconductors ranging from polarized light detection, spectral detection, and angle-sensing detection to self-powered detection is summarized.
3 The existing problems and perspectives are discussed which can inspire more researchers to rationally design new perovskite materials and micro/nano-structure for high-performance multifunctional photodetectors.

Keywords

Perovskite materials Crystal structure design Micro/nano-structure manipulation Working mechanism Multifunctional photodetectors
Zhao, Yingjie, Xing Yin, Pengwei Li, Ziqiu Ren, Zhenkun Gu, Yiqiang Zhang, and Yanlin Song. 2023. “Multifunctional Perovskite Photodetectors: From Molecular-Scale Crystal Structure Design to Micro/Nano-Scale Morphology Manipulation”. Nano-Micro Letters 15 (July):187. https://doi.org/10.1007/s40820-023-01161-y.
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