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Vol. 14 (2022)

Vertically Aligned Silicon Carbide Nanowires/Boron Nitride Cellulose Aerogel Networks Enhanced Thermal Conductivity and Electromagnetic Absorbing of Epoxy Composites

https://doi.org/10.1007/s40820-022-00863-z
Duo Pan
Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education; National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, People’s Republic of China
Gui Yang
Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education; National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, People’s Republic of China
Hala M. Abo‑Dief
Department of Chemistry, College of Science, Taif University, P. O. Box 11099, Taif 21944, Saudi Arabia
Jingwen Dong
Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education; National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, People’s Republic of China
Fengmei Su
Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education; National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, People’s Republic of China
Chuntai Liu
Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education; National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, People’s Republic of China
Yifan Li
Mechanical and Construction Engineering, Faculty of Engineering and Environment, Northumbria University, Newcastle upon Tyne NE1 8ST, UK
Ben Bin Xu
Mechanical and Construction Engineering, Faculty of Engineering and Environment, Northumbria University, Newcastle upon Tyne NE1 8ST, UK
Vignesh Murugadoss
Integrated Composites Laboratory (ICL), Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA
Nithesh Naik
Department of Mechanical and Manufacturing Engineering, Manipal Institute of Technology, Manipal Academy of Higher Education, Manipal, Karnataka 576104, India
Salah M. El‑Bahy
Department of Chemistry, Turabah University College, Taif University, P. O. Box 11099, Taif 21944, Saudi Arabia
Zeinhom M. El‑Bahy
Department of Chemistry, Al-Azhar University, Nasr City, Cairo 11884, Egypt
Minan Huang
Integrated Composites Laboratory (ICL), Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA
Zhanhu Guo
Integrated Composites Laboratory (ICL), Department of Chemical and Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA

Corresponding Author: Zhanhu Guo

zguo10@utk.edu

Nano-Micro Letters, Vol. 14 (2022), Article Number: 118

Abstract

With the innovation of microelectronics technology, the heat dissipation problem inside the device will face a severe test. In this work, cellulose aerogel (CA) with highly enhanced thermal conductivity (TC) in vertical planes was successfully obtained by constructing a vertically aligned silicon carbide nanowires (SiC NWs)/boron nitride (BN) network via the ice template-assisted strategy. The unique network structure of SiC NWs connected to BN ensures that the TC of the composite in the vertical direction reaches 2.21 W m−1 K−1 at a low hybrid filler loading of 16.69 wt%, which was increased by 890% compared to pure epoxy (EP). In addition, relying on unique porous network structure of CA, EP-based composite also showed higher TC than other comparative samples in the horizontal direction. Meanwhile, the composite exhibits good electrically insulating with a volume electrical resistivity about 2.35 × 1011 Ω cm and displays excellent electromagnetic wave absorption performance with a minimum reflection loss of − 21.5 dB and a wide effective absorption bandwidth (< − 10 dB) from 8.8 to 11.6 GHz. Therefore, this work provides a new strategy for manufacturing polymer-based composites with excellent multifunctional performances in microelectronic packaging applications.


Highlights:


1 Cellulose aerogel with vertically oriented structure was obtained by constructing a vertically aligned SiC nanowires/BN network via the ice template assisted strategy.
2 The thermal conductivity of the composite in the vertical direction reaches 2.21 W m−1 K−1 at a low hybrid filler loading of 16.69 wt%, which was increased 890% compared to pure epoxy.
3 The composite exhibits good electrically insulating with a volume electrical resistivity about 2.35×1011 Ω cm, and displays excellent electromagnetic wave absorption performance.

Keywords

Epoxy Ice template Vertical alignment Thermal conductivity Multifunctionality
Pan, Duo, Gui Yang, Hala M. Abo‑Dief, Jingwen Dong, Fengmei Su, Chuntai Liu, Yifan Li, Ben Bin Xu, Vignesh Murugadoss, Nithesh Naik, Salah M. El‑Bahy, Zeinhom M. El‑Bahy, Minan Huang, and Zhanhu Guo. 2022. “Vertically Aligned Silicon Carbide Nanowires/Boron Nitride Cellulose Aerogel Networks Enhanced Thermal Conductivity and Electromagnetic Absorbing of Epoxy Composites”. Nano-Micro Letters 14 (April):118. https://doi.org/10.1007/s40820-022-00863-z.
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