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Vol. 16 (2024)

Correction: Surface Patterning of Metal Zinc Electrode with an In-Region Zincophilic Interface for High-Rate and Long-Cycle-Life Zinc Metal Anode

https://doi.org/10.1007/s40820-024-01377-6
Tian Wang
Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, Yongin‑si, Gyeonggi‑do 17104, Republic of Korea
Qiao Xi
Frontiers Science Center for Flexible Electronics (FSCFE) and Shaanxi Institute of Flexible Electronics (SIFE), Northwestern Polytechnical University (NPU), 127 West Youyi Road, Xi’an 710072, People’s Republic of China
Kai Yao
Institute of Energy and Climate Research: Materials Synthesis and Processing (IEK‑1), Forschungszentrum Jülich GmbH, 52425 Jülich, Germany
Yuhang Liu
Frontiers Science Center for Flexible Electronics (FSCFE) and Shaanxi Institute of Flexible Electronics (SIFE), Northwestern Polytechnical University (NPU), 127 West Youyi Road, Xi’an 710072, People’s Republic of China
Hao Fu
School of Chemical Engineering, Sungkyunkwan University, 2066 Seobu‑Ro, Jangan‑Gu, Suwon‑si, Gyeonggi‑do, Republic of Korea
Venkata Siva Kavarthapu
Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, Yongin‑si, Gyeonggi‑do 17104, Republic of Korea
Jun Kyu Lee
Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, Yongin‑si, Gyeonggi‑do 17104, Republic of Korea
Shaocong Tang
Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, Yongin‑si, Gyeonggi‑do 17104, Republic of Korea
Dina Fattakhova‑Rohlfing
Institute of Energy and Climate Research: Materials Synthesis and Processing (IEK‑1), Forschungszentrum Jülich GmbH, 52425 Jülich, Germany
Wei Ai
Frontiers Science Center for Flexible Electronics (FSCFE) and Shaanxi Institute of Flexible Electronics (SIFE), Northwestern Polytechnical University (NPU), 127 West Youyi Road, Xi’an 710072, People’s Republic of China
Jae Su Yu
Department of Electronics and Information Convergence Engineering, Institute for Wearable Convergence Electronics, Kyung Hee University, Yongin‑si, Gyeonggi‑do 17104, Republic of Korea

Corresponding Author: Jae Su Yu

jsyu@khu.ac.kr

Nano-Micro Letters, Vol. 16 (2024), Article Number: 137

Abstract

The undesirable dendrite growth induced by non-planar zinc (Zn) deposition and low Coulombic efficiency resulting from severe side reactions have been long-standing challenges for metallic Zn anodes and substantially impede the practical application of rechargeable aqueous Zn metal batteries (ZMBs). Herein, we present a strategy for achieving a high-rate and long-cycle-life Zn metal anode by patterning Zn foil surfaces and endowing a Zn-Indium (Zn-In) interface in the microchannels. The accumulation of electrons in the microchannel and the zincophilicity of the Zn-In interface promote preferential heteroepitaxial Zn deposition in the microchannel region and enhance the tolerance of the electrode at high current densities. Meanwhile, electron aggregation accelerates the dissolution of non-(002) plane Zn atoms on the array surface, thereby directing the subsequent homoepitaxial Zn deposition on the array surface. Consequently, the planar dendrite-free Zn deposition and long-term cycling stability are achieved (5,050 h at 10.0 mA cm−2 and 27,000 cycles at 20.0 mA cm−2). Furthermore, a Zn/I2 full cell assembled by pairing with such an anode can maintain good stability for 3,500 cycles at 5.0 C, demonstrating the application potential of the as-prepared ZnIn anode for high-performance aqueous ZMBs.


Highlights:
1 A stable Zn anode was obtained by patterning Zn foil surfaces and endowing a zincphilic interface in microchannels.
2 The accumulation of electrons in the microchannel and the zincphilic interface promoted preferential heteroepitaxial Zn deposition in the microchannel region and subsequent homoepitaxial Zn deposition on the array surface.
3 The Zn symmetrical cells could undergo repeated plating/stripping for more than 25,000 cycles at the current densities of 10 and 20 mA cm−2.

Keywords

Zn metal anode Surface patterning Directional Zn deposition Aqueous Zn-I2 batteries
Wang, Tian, Qiao Xi, Kai Yao, Yuhang Liu, Hao Fu, Venkata Siva Kavarthapu, Jun Kyu Lee, Shaocong Tang, Dina Fattakhova‑Rohlfing, Wei Ai, and Jae Su Yu. 2024. “Correction: Surface Patterning of Metal Zinc Electrode With an In-Region Zincophilic Interface for High-Rate and Long-Cycle-Life Zinc Metal Anode”. Nano-Micro Letters 16 (February):137. https://doi.org/10.1007/s40820-024-01377-6.
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