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Vol. 10 No. 4 (2018)

Bi Nanoparticles Anchored in N-Doped Porous Carbon as Anode of High Energy Density Lithium Ion Battery

https://doi.org/10.1007/s40820-018-0209-1
Yaotang Zhong
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Bin Li
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Shumin Li
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Shuyuan Xu
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Zhenghui Pan
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Qiming Huang
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Lidan Xing
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China
Chunsheng Wang
Department of Chemical and Bimolecular Engineering, University of Maryland, College Park, College Park, MD 20740, USA
Weishan Li
School of Chemistry and Environment, South China Normal University, Guangzhou 510006, People’s Republic of China

Corresponding Author: Weishan Li

liwsh@scnu.edu.cn

Nano-Micro Letters, Vol. 10 No. 4 (2018), Article Number: 56

Abstract

A novel bismuth–carbon composite, in which bismuth nanoparticles were anchored in a nitrogen-doped carbon matrix (Bi@NC), is proposed as anode for high volumetric energy density lithium ion batteries (LIBs). Bi@NC composite was synthesized via carbonization of Zn-containing zeolitic imidazolate (ZIF-8) and replacement of Zn with Bi, resulting in the N-doped carbon that was hierarchically porous and anchored with Bi nanoparticles. The matrix provides a highly electronic conductive network that facilitates the lithiation/delithiation of Bi. Additionally, it restrains aggregation of Bi nanoparticles and serves as a buffer layer to alleviate the mechanical strain of Bi nanoparticles upon Li insertion/extraction. With these contributions, Bi@NC exhibits excellent cycling stability and rate capacity compared to bare Bi nanoparticles or their simple composites with carbon. This study provides a new approach for fabricating high volumetric energy density LIBs.


Highlights:


1 The Bi nanoparticles anchored in N-doped porous carbon (Bi@NC) composite was prepared by a facile replacement reaction method, in which ultrasmall Bi nanoparticles were homogeneously encapsulated in the carbon matrix
2 The N-doped carbon matrix enhanced the electric conductivity and alleviated the mechanical strain of Bi nanoparticles on Li insertion/extraction due to the larger void space, and Bi@NC exhibits excellent cyclic stability and rate capability for LIBs
3 The strategy developed in this work solves the cyclic instability issue of bismuth as anode for LIBs and provides a new approach to improve high volumetric energy density for electrochemical energy storage devices.

Keywords

Porous N-doped carbon Bi nanoparticles Anode Lithium-ion battery High energy density
Zhong, Yaotang, Bin Li, Shumin Li, Shuyuan Xu, Zhenghui Pan, Qiming Huang, Lidan Xing, Chunsheng Wang, and Weishan Li. 2018. “Bi Nanoparticles Anchored in N-Doped Porous Carbon As Anode of High Energy Density Lithium Ion Battery”. Nano-Micro Letters 10 (4):56. https://doi.org/10.1007/s40820-018-0209-1.
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