Issue

Vol. 16 (2024)

Multifunctional MXene/Carbon Nanotube Janus Film for Electromagnetic Shielding and Infrared Shielding/Detection in Harsh Environments

https://doi.org/10.1007/s40820-024-01431-3
Tufail Hassan
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Aamir Iqbal
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Byungkwon Yoo
Department of Materials Science and Engineering, Soongsil University, Seoul 06978, Republic of Korea
Jun Young Jo
Institute of Advanced Composite Materials, Korea Institute of Science and Technology, 92 Chudong‑ro, Bongdong‑eup, Wanju‑gun, Jeollabuk‑do 55324, Republic of Korea
Nilufer Cakmakci
Department of Materials Science and Engineering, Soongsil University, Seoul 06978, Republic of Korea
Shabbir Madad Naqvi
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Hyerim Kim
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Sungmin Jung
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Noushad Hussain
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Ujala Zafar
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Soo Yeong Cho
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Seunghwan Jeong
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea
Jaewoo Kim
Institute of Advanced Composite Materials, Korea Institute of Science and Technology, 92 Chudong‑ro, Bongdong‑eup, Wanju‑gun, Jeollabuk‑do 55324, Republic of Korea
Jung Min Oh
R&D Center INNOMXENE Co., Ltd., Daejeon 34365, Republic of Korea
Sangwoon Park
R&D Center INNOMXENE Co., Ltd., Daejeon 34365, Republic of Korea
Youngjin Jeong
Department of Materials Science and Engineering, Soongsil University, Seoul 06978, Republic of Korea
Chong Min Koo
School of Advanced Materials Science and Engineering, Sungkyunkwan University, Seobu‑ro 2066, Jangan‑gu, Suwon‑si, Gyeonggi‑do 16419, Republic of Korea

Corresponding Author: Chong Min Koo

chongminkoo@skku.edu

Nano-Micro Letters, Vol. 16 (2024), Article Number: 216

Abstract

Multifunctional, flexible, and robust thin films capable of operating in demanding harsh temperature environments are crucial for various cutting-edge applications. This study presents a multifunctional Janus film integrating highly-crystalline Ti3C2Tx MXene and mechanically-robust carbon nanotube (CNT) film through strong hydrogen bonding. The hybrid film not only exhibits high electrical conductivity (4250 S cm−1), but also demonstrates robust mechanical strength and durability in both extremely low and high temperature environments, showing exceptional resistance to thermal shock. This hybrid Janus film of 15 μm thickness reveals remarkable multifunctionality, including efficient electromagnetic shielding effectiveness of 72 dB in X band frequency range, excellent infrared (IR) shielding capability with an average emissivity of 0.09 (a minimal value of 0.02), superior thermal camouflage performance over a wide temperature range (− 1 to 300 °C) achieving a notable reduction in the radiated temperature by 243 °C against a background temperature of 300 °C, and outstanding IR detection capability characterized by a 44% increase in resistance when exposed to 250 W IR radiation. This multifunctional MXene/CNT Janus film offers a feasible solution for electromagnetic shielding and IR shielding/detection under challenging conditions.


Highlights:
1 A multifunctional Janus film is fabricated by integrating highly-crystalline and oxidation-resistant Ti3C2Tx MXene with carbon nanotube (CNT) film through strong hydrogen bonding, which exhibits high electrical conductivity of 4250 S cm−1 and robust mechanical strength of 77 MPa.
2 The MXene/CNT Janus film of 15 μm thickness demonstrates efficient electromagnetic interference shielding of 72 dB, low infrared (IR) emissivity of 0.09 and hence superior thermal camouflage performance, and outstanding IR detection capability, while maintaining its integrity equally at room temperature as well as under extreme conditions.
3 This multifunctional MXene/CNT Janus film offers a practical solution for electromagnetic shielding and IR shielding/detection in challenging conditions.

Keywords

MXene/carbon nanotube Janus film Electromagnetic interference shielding Infrared shielding Thermal camouflage Infrared detection
Hassan, Tufail, Aamir Iqbal, Byungkwon Yoo, Jun Young Jo, Nilufer Cakmakci, Shabbir Madad Naqvi, Hyerim Kim, Sungmin Jung, Noushad Hussain, Ujala Zafar, Soo Yeong Cho, Seunghwan Jeong, Jaewoo Kim, Jung Min Oh, Sangwoon Park, Youngjin Jeong, and Chong Min Koo. 2024. “Multifunctional MXene/Carbon Nanotube Janus Film for Electromagnetic Shielding and Infrared Shielding/Detection in Harsh Environments”. Nano-Micro Letters 16 (June):216. https://doi.org/10.1007/s40820-024-01431-3.
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